Zr-based MOFs: relation between linkers connectivity, stability, and catalytic activity

Metal–organic frameworks (MOFs) are widely researched but applied only in few commercial processes among others due to unknown stability. This study evaluates the stability of four zirconium-based MOFs with different linkers in water at pH 3.0 to 11.0. Results indicate that MOFs with tetratopic linkers (PCN-222, MIP-200) are more stable than those with ditopic or tritopic linkers (UiO-66, MOF-808), with MIP-200 being the most stable despite minor structural changes allowing thermal recrystallization.

https://pubs.rsc.org/en/Content/ArticleLanding/2024/QI/D4QI01366B

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